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戴翼虎和杨艳辉课题组在J. Energy Chem.上发表研究论文
 添加时间:2021/05/14 发布:

Tuned selectivity and enhanced activity of CO2 methanation over Ru catalysts by modified metal–carbonate interfaces

Qiaojuan Wanga, Yating Gaoa, Chantsalmaa Tumurbaatara, Tungalagtamir Boldb, Fei Weic, Yihu Daia,*, Yanhui Yanga,*

aInstitute of Advanced Synthesis, School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, Jiangsu, China

bSchool of Applied Sciences, Mongolian University of Science and Technology, Ulaanbaatar 14191, Mongolia

cBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua University, Beijing 100084, China

 

Abstract:

Ru/MnCO3 catalyst with metal-carbonates interfaces exhibits superior catalytic selectivity and anti-CO stability in CO2 methanation in comparison with Ru/MnO catalyst, benefiting from enhanced CO2 and H2 dissociation, formation of active Ru–CO* intermediates, and further rapid transformation into CH4.

 

Journal of Energy Chemistry 64 (2022) 38–46.

(中国科技期刊卓越行动计划重点期刊,影响因子:7.216)

 

论文链接: https://doi.org/10.1016/j.jechem.2021.04.039

 

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